Cloud-Base Distribution and Cirrus Properties Based on Micropulse Lidar Measurements at a Site in Southeastern China

Jianjun LIU,Zhanqing LI,ZHENG Youfei,and Maureen CRIBB

1State Laboratory of Earth Surface Process and Resource Ecology and College of Global Change and Earth System Science, Beijing Normal University,Beijing 100875

2Earth System Science Interdisciplinary Center,University of Maryland,College Park,Maryland,20740,USA

3Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Nanjing University of Information Science and Technology,Nanjing 210044

Cloud-Base Distribution and Cirrus Properties Based on Micropulse Lidar Measurements at a Site in Southeastern China

Jianjun LIU1,2,3,Zhanqing LI?1,2,ZHENG Youfei3,and Maureen CRIBB2

1State Laboratory of Earth Surface Process and Resource Ecology and College of Global Change and Earth System Science, Beijing Normal University,Beijing 100875

2Earth System Science Interdisciplinary Center,University of Maryland,College Park,Maryland,20740,USA

3Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Nanjing University of Information Science and Technology,Nanjing 210044

The cloud fraction(CF)and cloud-base heights(CBHs),and cirrus properties,over a site in southeastern China from June 2008 to May 2009,are examined by a ground-based lidar.Results show that clouds occupied the sky 41%of the time. Signif i cant seasonal variations in CF were found with a maximum/minimum during winter/summer and similar magnitudes of CF in spring and autumn.A distinct diurnal cycle in the overall mean CF was seen.Total,daytime,and nighttime annual mean CBHs were 3.05±2.73 km,2.46±2.08 km,and 3.51±3.07 km,respectively.The lowest/highest CBH occurred around noon/midnight.Cirrus clouds were present～36.2%of the time at night with the percentage increased in summer and decreased in spring.Annual mean values for cirrus geometrical properties were 8.89±1.65 km,9.80±1.70 km,10.73±1.86 km and 1.83±0.91 km for the base,mid-cloud,top height,and the thickness,respectively.Seasonal variations in cirrus geometrical properties show a maximum/minimum in summer/winter for all cirrus geometrical parameters.The mean cirrus lidar ratio for all cirrus cases in our study was～25±17 sr,with a smooth seasonal trend.The cirrus optical depth ranged from 0.001 to 2.475,with a mean of 0.34±0.33.Sub-visual,thin,and dense cirrus were observed in～12%,43%,and 45% of the cases,respectively.More frequent,thicker cirrus clouds occurred in summer than in any other season.The properties of cirrus cloud over the site are compared with other lidar-based retrievals of midlatitude cirrus cloud properties.

cloud-base distribution,cirrus properties,lidar,southeastern China

1.Introduction

The signif i cant inf l uences of clouds on the redistribution of energy and moisture,atmospheric dynamics,thermodynamics,and the hydrological cycle on regional and global scales by means of scattering and absorbing radiation and releasing latent heat mainly depend on their spatio–temporal variations in vertical structure and horizontal distribution (Stephens,2005;Dong et al.,2005).Among the multiple cloud types,cirrus clouds play an important role in Earth’s climate and cover 17%–30%of Earth’s atmosphere(Dessler and Yang,2003;Sassen et al.,2008).The frequency of occurrence of cirrus clouds can reach 45%in the tropics (Stubenrauch et al.,2006).Cirrus clouds in the upper troposphere have two opposite effects:an infrared greenhouse effect and a solar albedo effect,which strongly depend on their macrophysical and optical properties.The radiative and climate effects of clouds,especially cirrus clouds,still remain largelyuncertain.A clear understandingof their macrophysical and optical propertiesat differentgeographicallocations is essential for climate modeling studies(Giannakaki et al.,2007).Satellite-based passive remote sensing,such as that performedby the ModerateResolution ImagingSpectroradiometer(MODIS),has enabled the observation of cloud characteristics such as the amount and top height on a global scale(Platnicketal.,2003).However,theirretrievalaccuracy suffers from various limitations(Chang and Li,2005).Passive satellite sensors with visible and near-infrared channels have diff i culty inferring the properties of low and optically thin clouds(Wu et al.,2009).Spaceborne active remote sensors,such as CloudSat and Cloud-Aerosol Lidar Pathf i nder Satellite Observations(CALIPSO),can provide information aboutcloudverticalstructureworldwide(Winkeret al.,2003; Mace et al.,2009),but the temporal resolution is limited, making any investigation of the diurnal cycle of clouds over specif i c regions impossible(Min et al.,2010).

Ground-based instruments can capture the diurnal cycleof clouds and are valuable for monitoring long-term trends at fi xed locations.Although ground-based lidars cannot penetrate optically thick clouds or determine cloud-top heights, they can detect the presence of clouds and measure lowest layer cloud-base heights(CBH).Numerous studies have demonstratedtheirabilityto observecloudproperties(Campbell and Shiobara,2008;Shupe et al.,2011;Thorsen et al., 2013),and in particular,to quantify and characterize the vertical structure and optical properties of cirrus clouds.Lidar observations provide information on cloud vertical structure with a much higher sensitivity to optically thin clouds than a cloud radar(Thorsen et al.,2013).The capability of a ground-based lidar system to detect thin cirrus clouds makes it one of the most appropriateinstrumentsto use for the study of these clouds(Noel et al.,2007).

Using ground-based lidar data,many studies have been carried out regarding the temporal and spatial variations of cloud structure(Maheshet al.,2005;Bissonnette et al.,2007; Shupe et al.,2011)and macro-and microphysicaland optical properties,as well as radiative effects of cirrus clouds over different regions,such as the tropics(Sassen and Campbell, 2001;Comstock et al.,2002;Seifert et al.,2007;Sunilkumar et al.,2008)and the midlatitudes(Reichardt,1999;Keckhut et al.,2005;Wang et al.,2008;Das et al.,2009;Dupontet al., 2010).Signi fi cant differences in cloud characteristics exist from one region to another and the representation of clouds in climate models is still poor(Zhang et al.,2005).Characterizing the spatial and temporal distributions of clouds with better spatial and temporal resolutions,including the macrophysics and optical properties of cirrus clouds at different geographic locations,is fundamental to understanding and quantifying the roles of clouds in climate change and in improving weather climate models(IPCC,2007;Vukicevic et al.,2010).

During the deployment of the United States Department ofEnergy’sAtmosphericRadiationMeasurementMobileFacility in China(Li et al.,2011),extensivemeasurementswere made at Taihu from May 2008 to December 2009 for the purpose of studying aerosol–cloudinteractions under heavily polluted conditions.The site(31.702°N,120.358°E;10 m above sea level)is located in the heart of the Yangtze Delta, where there is an abundance of different types of anthropogenic aerosols(Li et al.,2007).To help unravel aerosol–cloud interactions,cloud and aerosol properties were measured by numerousadvancedinstruments installed at the site. By virtue of continuous ground-based lidar measurements, we investigate the cloud-base distribution and geometrical and optical properties of cirrus clouds with the goal of laying the foundations for studying aerosol–cloud interactions.

The remainder of the paper is organized as follows.Section 2 describes the micropulse lidar system and methods used to determine the cloud mask and to retrieve cirrus optical properties.Seasonal patterns and the diurnal cycle of the cloud-base distribution are discussed in section 3.Section 4 presents the seasonal evolution of the vertical structure,macrophysical properties,and optical properties of cirrus clouds.Section 5 gives the main conclusions.

2.Instruments and methods

Adepolarization-sensitive micropulselidar(MPL), which is a compact and solid state lidar developed at NASA and manufacturedby the Sigma Space Corporation,was used (Spinhirne et al.,1995).It uses an Nd:YLF pulsed laser diode,operating at a wavelength of 527 nm with a pulse repetition rate of 2500 Hz.The bin time of the MPL receiver was 200 ns,with a 30 m vertical resolution.The MPL system averages many low-energy pulses in short durations to achieve a good signal-to-noise ratio(SNR).A pulsed solidstate laser,a narrow f i eld-of-view(FOV:～100μrad),narrow interference f i lters(～0.3 nm full width at half maximum), and photon counting capability result in a highly sensitive instrument.Further detail regarding the features of the MPL can be found in Spinhirne et al.(1995).

Figure 1 shows the steps taken to retrieve cloud properties in this study.Using the methoddescribed by Campbell et al.(2002),raw data were corrected to the normalized relative backscattersignal(NRB).Lidarsignalsat upper-tropospheric ranges are signif i cantly inf l uenced by the afterpulse.To minimize this inf l uence,afterpulse calibrations were performed frequently using the methods proposed by Campbell et al. (2002)and Liu et al.(2011).Cloud boundaries were derived using the cloud mask algorithm of Wang and Sassen (2001).This algorithm is based on characteristics of the lidar signal,as in the differential zero-crossing and threshold methods,and also takes into account the underlying physical differences between cloud and aerosol layers,and noise effects.To distinguish a cloud layer from an aerosol layer, empirical threshold values were used(Clothiaux et al.,1998; Campbell et al.,2002;Zhao et al.,2014).Use of these values in the algorithm proved successful at separating clouds from aerosolswithhighaccuracy.MoredetailisgiveninWangand Sassen(2001).Cirrus optical properties were retrieved using the algorithmof ComstockandSassen(2001),whichis based on the solution of the lidar equation.The cloud backscatter coeff i cient,βc(km sr?1),is given by

whereβmis the scattering contribution from air molecules,S(z)is the normalized lidar backscatter signal,andηandkare the forward multiple-scattering correction parameter and the extinction-to-backscatter ratio,respectively.z0denotes the height just below the cloud base where the scattering is presumably due to molecules,andzis the height at which the backscatter signals are received.The parameterkis determined using an iterative technique where the value ofkis increased incrementally from 5 to 100 sr.It reaches its f inal value when the average backscatter coeff i cient above the cloud is equal to the average molecular backscatter coeff icient above the cloud.

The optical depth of the cirrus cloud,τc,can be determined by integratingβcbetween the cirrus cloud base,zb, and the cloud top,zt.The primary uncertainty in theτcretrieval is in estimating the parameterk,which results in a maximum uncertainty of～24%for the retrieved value ofτc(Comstock and Sassen,2001).This algorithm has been applied to several long-term datasets in both the midlatitudes and the tropics with reasonable accuracy(Sassen and Comstock,2001;Comstock et al.,2002).The forward multiplescattering correction parameter was used to compensate for the effect of forward multiple-scatteringon the return energy. The contribution of forward multiple-scattering to the total cloud optical depth was assumed to be relatively small here because the MPL receiving telescope has a narrow FOV(Das et al.,2009).In this study,we setη=0.9 based on simulations ofthe multiplescatteringcorrectionfactorby Comstock and Sassen(2001).

The linear volume depolarization ratio(δ),def i ned as the ratio of cross-polarizedand co-polarizedscattering ratios, was computed from MPL measurements using the method of Flynn et al.(2007).This quantity is useful for studying the shape of ice crystals and provides dynamical information about cloud formation.

3.Cloud fraction and cloud-base distribution

3.1.Cloud fraction

The cloud fraction(CF)is de fi ned here as the percentage of returns that are identi fi ed as cloudy within a specifi ed sampling period(e.g.,a month)regardless of the number of cloud layers.Although lidar-derived CF represents only a pencil beam of the sky that depends on the advection of clouds overhead,studies have found that they are statistically representative in terms of long-term averages(Dong et al., 2006,2010).

Figure 2a shows the monthly mean CF from June 2008 to May 2009 with seasonal and annual mean values summarized in Table 1.CF varied signif i cantly throughout the year. CF peaked during February,October and March,with values larger than 50%and reached a minimum during June and July,with values around 25%.The largest CF(～67.2%)was more than 2.5 times greater than the smallest CF(25.4%). The annual averaged CF was 40.6%and the seasonal mean CF was marked by maxima during winter and minima during summer(Table 1).The CF seasonal variability ref l ects the difference in large-scale atmospheric dynamics between the summer and the winter and transition periods(Kollias et al.,2007).A similar CF and the same seasonal variation in CF were also found at another midlatitude site,the Southern Great Plains(SGP)site in the U.S.(Dong et al., 2006).Monthly(Fig.2b)and seasonal(Table 1)mean daytime and nighttime CF show that more clouds occurred during the night than during the day.On average,the largest seasonal CF for daytime and nighttime occurred in winter and spring,and the smallest values for both were found in summer.Annual mean daytime and nighttime CFs were 17.9% and 22.7%,respectively,during the entire study period.

Seasonal and annual mean diurnal cycles of the CF anomaly,def i ned as the difference between hourly and daily mean CF,are presented in Fig.3.The annual average CF anomaly experienced a signif i cant diurnal cycle with amplitudes of about 24.6%.The annual average CF anomaly decreased sharply from the beginning of the day to midday,and then gradually increased again.Maxima in the CF anomaly occurredat around 0200 and 2200 LST and the minimum occurred at around local noon.This is possibly related to an increase in solar heating at the cloud top at noon resulting in a relative stabilization of the cloud layer leading to somewhat less cloudiness(Shupe et al.,2011).Concerning the seasonal diurnal cycle,a strong diurnalvariation can be seen in spring, summer,and autumn with amplitudes of 35.0%,32.1%,and 24.2%,respectively.A relatively moderate diurnal variation was found in winter with amplitude of about 15.7%,which is partly due to the weak local convection at the surface in wintertime(Dong et al.,2005).Generally speaking,seasonal patterns in the variation of the diurnal CF mean anomaly are similarto theannualpattern,exceptforwintertime.Inwinter, the minimum CF mean anomaly occurred at 0500 LST and around 1200 LST,with a sharp variation between the beginning of the day and the late afternoon,followed by a leveling offfortheremainderofthenight.Althoughsimilarvariations are found in spring,summer and autumn,differences in the relative variation are seen.For example,in summer,the variation was smoother before and after noon than it was during spring and autumn.

3.2.Cloud-base distribution

Due to the severe attenuation in lidar signals by thick clouds,theanalysisofcloudbases presentedherereferstothe analysis of the f i rst cloud layer base detected fromthe ground regardless of the number of cloud layers above it.Monthly statistics of total(T),daytime(D),and nighttime(N)CBH, with annual means given on the right-hand side of the plot (shaded),are summarized in Fig.4.Seasonal and annual means,standard deviations,and median values of CBH for T, D,and N cases are shown in Table 1.Relatively high annual meanCBHs werefound,withmeanvaluesof3.05±2.73(T), 2.46±2.08(D),and 3.51±3.07km(N).The highest annual mean CBH was found during the night.Monthly variations in the mean CBH for all cases were almost the same,with thehighest values in the spring and summer,and especially duringthenighttimeperiod(Table1).Becausemonthly/seasonal distributions of CBH are strongly skewed towards higher values,monthly/seasonal median values are typically lower,although the same general trends are seen(Shupe et al.,2011). Similar seasonal patterns in CBH,i.e.,maximum/minimum values in summer/winter,have been found at other sites,e.g., the SGP site(Dong et al.,2005),the South Pole(Mahesh et al.,2005),and Eureka in the Arctic(Shupe et al.,2011).

Table 1.Seasonal and annual mean cloud fraction(CF)and cloud-base height(CBH)in three altitude bins(L,M,H)*based on total(T), daytime(D),and nighttime(N)observations.Also included are the seasonal and annual mean probability distribution functions(PDFs)in the three altitude bins.

Probability distribution functions(PDFs)of monthly and annual mean CBH,given in 0.5 km vertical range bins,are shown in Fig.5.Seasonal and annual mean PDFs for three different altitude ranges(below 2 km,2–5 km,and above 5 km)are listed in Table 1.Looking at the annual mean vertical distribution,the largest number of detected cloud bases (～17%)falls within the surface-based temperature inversion (0.5–1 km).A similar result was reported by Dong et al. (2005)at the SGP site.Annual mean vertical probability distributions graduallydecrease with increasing height above 1 km.Annual mean PDFs of CBH within the three height ranges were about 48.9%,30.3%,and 20.8%,respectively (Table 1).

The monthly and annual diurnal cycles of mean CBH are plotted in Fig.6.CBHs were averaged over a half-hour period in this study.The diurnal cycle of CBH in summer and spring varied greatly throughout the day.CBHs hit a minimum around noonand reached a maximum aroundmidnight. The strongest signatures were seen in July.The highest CBH occurred from 0030 to 0100 LST and the lowest CBH occurred between 1100 and 1130 LST.The difference between the highest and lowest CBH was 5.1 km.The daily range in CBH during autumn and winter was not as dramatic.For example,in February,changesin CBH throughoutthe day were less than 1.1 km.The diurnal cycle in CBH was weak in autumn and in winter.The annual diurnal cycle in mean CBH (Fig.6b)hasthesamefeaturesasthevariationinCBH during spring and summer.From 0300 to 1000 LST,a marked decrease in CBH occurred,and from 1700 to 2100 LST a sharp increase was seen.

4.Cirrus cloud properties

To differentiate between water clouds and cirrus clouds, the following three criteria are used to identify cirrus clouds: (1)CBH is greater than 7 km;(2)δis greater than 0.03 (Das et al.,2010);and(3)the maximumτcis less than 3.0 (Sassen and Campbell,2001).Only nighttime data are used here because,during the day,the signal-to-noise ratio is poor at high altitudes due to contamination by background photon counts(Dupont et al.,2011).The cirrus occurrence fraction is def i ned as the ratio of the number of nights that cirrus was detected to the total number of nights measurements were made.Cirrus clouds were identif i ed in 42,45,17,and 13 nights out of a total of 83,87,85,and 68 nights during spring,summer,autumn,and winter,respectively.This corresponds to cirrus occurrence fractions of 50.6%,51.7%, 20%,and 19.1%,respectively.The annual mean cirrus occurrence fraction was 36.2%.A maximum cirrus occurrence in summer and a minimum in winter were also found from two years’worth of Cloud-Aerosol Lidar with Orthogonal Polarization(CALIOP)data over northern China(Min et al., 2011).The summertime maximum happens because there is a relatively abundant supply of upper-tropospheric water vapor introduced by regional convective activity inf l uenced by the western tropical Pacif i c and because of the seasonal meridional displacement of subtropical cirrus bands(Sassen et al.,2008;Min et al.,2011).The annual mean cirrus occurrence in our study is similar to that(37%)calculated from an eight-year cirrus climatology generated by Das et al.(2009) over Chung-Li,a site in East Asia.

4.1.Cirrus geometrical properties

Figure 7 shows the following cirrus geometrical properties in the form of box plots:(a)CBH,(b)mid-cloud height; (c)cloud-top height,and(d)geometrical thickness in each month and year-round.Seasonal and annual mean cirrus geometrical properties and vertical probability distributions of cirrus geometrical properties are summarized in Table 2 and plotted in Fig.8.The mid-cloudheight is the weighted CBH, which is def i ned as

Here,zbaseandztopcorrespond to CBH and CTH,respectively,andzis the height at which the backscatter signals are received.The parameterRB(z)is the backscattering ratio, which can be expressed as

whereβγ(z)andβc(z)are the backscattering coeff i cients of air and cloud at the laser wavelength,respectively.

Figures 7a and 7b show that cirrus base and mid-cloud heights varied greatly by month.Maximum and minimum monthly mean cirrus base(mid-cloud)heights of 10.8±2.2 km(11.8±2.2km)and 7.7±0.6km(8.4±0.6km)occurred in July and December,respectively.For most of the year, cloud-base and mid-cloud height distributions were strongly skewed towards higher values because median values were typically lower,although the same general trends are seen (Shupeet al.,2011).Seasonal meancirruscloud-baseheights (mid-cloud heights)were 8.38±1.02 km(9.21±0.99 km), 9.89±1.97 km(10.97±1.93 km),7.94±0.71 km(8.66± 0.69 km),and 7.75±0.60 km(8.40±0.61 km)in spring, summer,autumn,and winter,respectively,with an annual mean of 8.89±1.65 km(9.80±1.70 km)during the course of the study(Table 2).The vertical distribution of summertimecloud-baseheightsshowsabroaddistributioninsummer ranging from 7 km to 14.3 km and a relatively smooth variation with height.For other seasons,about 62.7%(spring), 82.8%(autumn)and 89.4%(winter)of cirrus cloud bases are located below 8.5 km.Figure 8b shows that the vertical occurrence of mid-cloud heights also experienced a smooth variation with height in summer,with peaks at 8.5 km and 12.5–13 km.In spring,around 81.5%of mid-cloud heights fell between 8.0 and 10.5 km,and about 87.5%and 93.0%of mid-cloud heights varied between 7.5 km and 9.5 km in autumn and winter.From data over the whole year,cirrus base andmid-cloudheightsrangedfrom7 kmto14.3km andfrom 7.1 km to 15 km,respectively.The majority of cirrus base heights(～56%)and mid-cloud heights(～50%)were located in the range of 7–8.5 km and 8–9.5 km,respectively.

Cirrus cloud-top heights(CTHs)also experienced significant monthly variations(Fig.7c).Mean CTHs were 10.08±1.07(spring),12.10±1.98(summer),9.25±0.80(autumn) and 8.99±0.75km(winter),with an annual mean of 10.73± 1.86 km.Figure 8c shows that CTHs had a broad(7–16 km) and multimodal distribution,with a major mode centered on the 13–13.5 km height range in summer.Nearly 70%and more than 90%of CTHs in spring and in autumn and winter, respectively,were located below 10.5 km.Most CTHs(more than 40%)reached an altitude of 9–10.5 km during the study period.

Table 2.Seasonal and annual averages,standard deviations,and median values of cirrus base height(BH),top height(TH),mid-height (MH),and geometrical thickness(GT).

Cirrus geometrical thickness monthly and annual statistics are shown in Fig.7d.There is a noticeable month-tomonth variation.Maximum(minimum)values are found in summer(autumn).The annual mean thickness was 1.83± 0.91 km and seasonal mean thicknesses were 1.69±0.76 (spring),2.22±0.97(summer),1.31±0.72(autumn),and 1.24±0.57 km(winter).The PDF for cirrus thickness in each season(Fig.8d)has a distribution with one mode and thicknesses are mostly less than 5 km(spring),6 km(summer),3.5 km(autumn)and 3 km(winter).Peaks in thickness werefoundin 26.1%ofthecases inspring(1.5–2km),23.8% of the cases in summer(2–2.5 km),22.0%of the cases in autumn(1–1.5 km),and 35.1%of the cases in winter(1–1.5 km).In terms of the annual PDF,approximately 86.2%of the cases studied had thicknesses between 0.5 km and 3 km.

4.2.Cirrus optical properties

Cirrus optical properties,including the extinction-tobackscatteringratio(commonlyknownasthelidarratio,LR), the cirrus extinction coeff i cient(σ),andτcover Taihu are investigated.In the case of sub-visible cirrus,the Fernald retrieval relation(Fernald,1984)is insensitive to estimates of LR.For such cases encountered in this study,the cirrus LR is set to 24 sr.This value represents the mean of all retrieved cirrus LR for clouds withτ＜0.3 found in the study. This approach has been used by Das et al.(2009).Mean LR in spring,summer,autumn,and winter was 27.6±20.1, 23.5±15.1,24.1±15.3,and 25.3±16.7 sr,respectively, with an annual mean LR of 25.3±17.7 sr(Table 3).Sassen et al.(1989)simulated the backscattering-to-extinction ratio (1/LR)for hexagonal ice crystals and found that for thinplate,thick plate,and column ice crystals,1/LR is equal to 0.026 sr?1,0.086 sr?1,and 0.038 sr?1,respectively.Figure 9a shows the frequency occurrence of 1/LR calculated from data collected over Taihu.About 70%of the values fall between 0.025 sr?1and 0.055 sr?1,with a peak at 0.035 sr?1,suggesting that most of the cirrus clouds observed in our study consisted of column ice crystals.Values of 1/LR close to 0.2 sr?1are likely due to specular ref l ection caused by falling or horizontally-oriented ice crystals,especially if observed through a vertically-pointing lidar(Ansmann et al., 1992;Das et al.,2009).Seasonal and annual mean LR as a function of mid-cloud height is shown in Fig.9b.The LR is averaged over every 1 km height bin and vertical bars represent the standard deviation of the annual mean LR.There is no obvious correlation between LR and mid-cloud heights. This may be due to large variations in ice crystal mode and size and is also likely due to the process that forms cirrus clouds over the site.

In this study,σranged from 0.001 to 1.59 km?1,with an annual mean of 0.25±0.31 km?1(Table 3).Seasonal meanσvalues were 0.23±0.35(spring),0.19±0.19(summer),0.37±0.56(autumn),and 0.20±0.40 km?1(winter). Meanσas a function of mid-cloud height in each season and over the entire study period is shown in Fig.10.The meanσis averaged over every 1 km height bin and the standard deviations of the annual meanσare shown as vertical bars.On the whole,the meanσdecreased with increasing mid-cloudheight in each season and year-round.Others have shown thatσincreases with mid-cloud temperature(Pace et al.,2003;Das et al.,2010),whichis consistentwiththis study because higher mid-cloud heights are usually associated with relatively lower temperatures.

For all cirrus cloud cases in this study,τcranged from 0.001 to 2.475,with mean values of 0.31±0.24,0.40±0.33, 0.34±0.30,and 0.20±0.20 in spring,summer,autumn,and winter,respectively.The annual mean was 0.34±0.33(Table 3).Clouds with differentτcplay different roles when it comes to cloud radiative effects,which depend on cloud composition and geometrical thickness.Cirrus clouds here are classif i ed into three cloud categories:sub-visible cloud (τc＜0.03),optically thin cloud(0.03＜τc＜0.3),and optically dense cloud(τc＞0.3)(Seifert et al.,2007;Das et al., 2009).Table 3 lists the optical properties of cirrus cloud in eachof these categoriesforall seasons andyear-round.Num-bers in parentheses are standard deviations.For all analyzed cirruscloudcases,～12%ofthecases were sub-visiblecirrus,～43%were thin cirrus,and 45%were dense cirrus.Signif icant differences in the magnitude ofσfor all three categories of cirrus cloud are found.

Table 3.Seasonal and annual mean optical properties of sub-visible,thin,and dense cirrus.Standard deviations are given in parentheses.

4.3.Comparisons with lidar-based retrievals

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Forthe sake ofa propercomparison,we summarizeinformation about midlatitude cirrus clouds detected by groundbased and space-bornelasers from studies made over the past decade(Table 4).A large range of cirrus CBH can occur. For example,at the Obs′ervatoire de Haute Provence(OHP) and Site Instrumental de Recherche par T′el′ed′etection Atmosph′erique(SIRTA)sites in France,they range from 7–13 km,and over the Clouds and the Earth’s Radiant Energy System(CERES)Ocean Validation Experiment(COVE)and SGP sites in the U.S.,cirrus CBH rangesfrom7 km to 15km(Dupont et al.,2010).In this study,cirrus CBH ranges from 7 km to 14 km.Mean cirrus base heights range from 8 to 10 km in most of the studies listed in Table 4.One site (Chung-Li)has a relatively high base height of greater than 12 km(Das et al.,2009).The mean base height from the studies presented in Table 4(excluding Chung-Li)is around 9.2 km,which is considered a typical base height for midlatitude cirrus clouds.The mean cloud-base height in this study(8.9±1.7 km)is comparable to this typical value.As listed in Table 4,mean cirrus cloud-top heights range from 9.5 km to 14.4 km,with most located around 11 km.The mean value(excluding Chung-Li)is about 11.0 km,which is closeto thevaluefoundinthis study(10.7±1.9km).A study on the global characterization of cirrus using CALIPSO data (not shown in Table 4)has also shown that,between 20°N and 60°N,cirrus clouds with base and top altitudes at 8 km and 11 km,respectively,occur most often and that there are no signi fi cant differences in the vertical distribution of cirrus clouds between(20°–60°N)and(20°–60°S)(Nazaryanet al., 2008).Althoughcloud thickness generallyhas a broaddistribution,e.g.,from about 7.0 km over Salt Lake City(Sassen and Comstock,2001)and Chung-Li(Das et al.,2009),and ranging from 0.5 km to 5 km over French and American sites(Dupont et al.,2010),most cirrus cloud thicknesses are less than 2.0 km.The mean cirrus thickness over Taihu was 1.83±0.91 km,which is slightly larger than that found over the OHP(Goldfarb et al.,2001),Prestwick and Punta Arenas(Immler and Schrems,2002),and SIRTA(Dupont et al., 2010)sites,andless thanthat overSalt Lake City(Sassen and Comstock,2001),Thessaloniki(Giannakakiet al.,2007),and BuenosAires(Lakkiset al.,2009).Averagingall valuesfrom Table 4,the typical thickness of midlatitude cirrus clouds is 1.7 km.Based on cirrus data sets derived using different detection techniques,Dowling and Radke(1990)reported that a typical global value for cirrus cloud thickness is 1.5 km.

The mean LR in this study was 25±17 sr for all cirrus cloud cases,which falls within the range of values shown in Table 4.Using lidar data from Salt Lake City,Sassen and Comstock(2001)calculated a mean LR of about 24±38 sr and a median value of～27 sr.They also reported that the mean LR for anvil cirrus,and cirrus formed from synoptic fl ows and from orographic effects,is～24±43 sr,26±40 sr,and 20±35 sr,respectively.The mean LR for midlatitude cirrus in the Northern Hemisphere over Thessaloniki from 2000 to 2006 was 30±17 sr(Giannakaki et al.,2007). FromtwostudiesmadeatChung-Li(Chenet al.,2002;Das et al.,2009),values of 29±12 sr and 23±16 sr were found,respectively.A similar value of 23 sr was found over Prestwick during September to October 2000(Immler and Schrems, 2002).At a site in the Southern Hemisphere,a mean value of 26 sr was calculated from data collected in March and April of 2000(Immler and Schrems,2002).Results found in this study are consistent with those from these earlier works.The LR depends on the properties of ice crystals and is also in fl uenced by the height of the cirrus cloud.For example,in the study over Chung-Li,the LR varied randomly below 12 km and varied between 20 sr to 40 sr from 12–15 km,and 10 sr to 30 sr from 15–16 km(Chen et al.,2002).

The variability inτcdepends on the composition and thickness of the cloud(Sivakumar et al.,2003).From the study by Sassen and Cho(1992),approximately 60%of cirrus clouds are optically thin and,over Chung-Li,more than 80%of the cirrus cases are optically thin(Das et al.,2009). Overall,most midlatitude cirrus clouds are optically thin and occur 60%of the time.The frequency of sub-visible cirrus in this study is approximately 12%,which is much higher than the 3%reported by Giannakaki et al.(2007)over Thessaloniki and the 5%reported by Dupont et al.(2010)over the SGP site.It is signif i cantly lower than the 38%reported by Das et al.(2009)over Chung-Li.The frequency of subvisible cirrus in this study is roughly in line with that from studies of midlatitude cirrus over the COVE site(Dupont et al.,2010),at the OHP(Goldfarb et al.,2001;Dupont et al., 2010),Salt Lake City(Sassen and Campbell,2001),Prestwick(ImmlerandSchrems,2002),PuntaArenas(Immlerand Schrems,2002),the SIRTA(Dupont et al.,2010)sites,and northernChina(Minet al.,2010).Sincemost midlatitudecirrus cloudsare opticallythin,the meanvalue ofτcis generally less than 1.0.The meanτfor all cirrus clouds in this study is 0.34±0.33,which is consistent with the mean values of 0.31 reported by Giannakaki et al.(2007)and 0.28 reported by Immler and Schrems(2002).However,the mean value found in this study is signif i cantly larger than the value of 0.16±0.27 reported by Das et al.(2009)and slightly smaller than the value of 0.41±0.68 reported by Min et al.(2011). The mean value ofτcis muchsmaller than that of 0.75±0.91 reported by Sassen and Campbell(2001).

These differences are expected due to the variability in cirruscloudsarisingfromfactorssuchassynopticconditions, water vapor amount,and number of cloud condensation nuclei(Sassen and Campbell,2001;Min et al.,2010).In addition,discrepancies may also arise from artifacts caused by instrument characteristics,such as lidar vertical resolution, maximum pulsed energy,receiver solid signals and so on,as well as from different methods used to retrieve optical properties and to correct for multiple scattering.Different ways of identifying/def i ning a cirrus cloud can also result in differences in their optical properties.For example,Das et al. (2009)def i ne a cirrus cloud as the lowest cloud with a base height located above 8 km,while Wang and Sassen(2001, 2002)and Dupont et al.(2010)use a value of 7 km for the lowest cirrus CBH.An even smaller value of 5 km was used in the studies by Nazaryan et al.(2008)and Min et al.(2010) usingCALIPSOdata.OtherobservedvariablessuchasRB(z) and lidar depolarization ratio can also be used to identify cirrus clouds.Discrepancies in any of these can contribute to differences in retrieved cirrus cloud properties.

5.Conclusion

Towards gaining insights into the characteristics of aerosols,clouds,and their interactions in southeastern China, a heavily polluted area in East Asia,a suite of instruments,including a depolarization-sensitive MPL,was installed at Taihu,located in the center of the Yangtze Delta region,from May 2008 to December 2009.The seasonal patterns and the diurnal cycles of CF and CBH,and the vertical structure and optical properties of cirrus clouds,were f i rst examined.Althoughonlyoneyear’sworthofdatawerecollected,theyprovide a useful f i rst look at the characteristics of clouds,especially cirrus clouds,over this part of the world.The measurements collected also provide the opportunity to make comparisons with similar clouds in other regions of the world.

Overall,clouds were observed 41%of the time over the site throughout the campaign,and varied seasonally with a typical summer minimum(27.7%)and a winter maximum (51.4%).These results are similar to those reported in a study based on ground-based radar-lidar observations over the SGP site from 1997 to 2002.In most months,more clouds were found at night than during the day.On average, the largest/smallest seasonal CF occurred in winter/summer during the day,while the largest/smallest value at night occurred in spring/summer.Annual average CF experienced a signif i cant diurnal cycle with amplitudes of about 24.6%. Cloud amounts decreased noticeably from the beginning of the day to midday,and then continuously increased from local noon to the end of the day.Annual mean CBHs were 3.05±2.73,2.46±2.08,and 3.51±3.07 km for all clouds, daytime clouds only,and nighttime clouds only,respectively. The highest CBHs were found in spring and summer,especially during the night.The largest number of detected cloud bases fell within the range of 0.5 km to 1.0 km.The annual mean diurnal cycle of CBH shows that low CBH occurred around noon and high CBHs appeared around midnight.The seasonal mean diurnal cycle of CBH was strong in spring and summer and relatively weak in autumn and winter.

Cirrus clouds comprised～36.2%of nighttime cloud observations with peaks in occurrence during the summer.Cirrus base heights ranged from 7 km to 14.3 km.More than 56%of cirrus base heights were located between 7 km and 8.5 km.Cirrus top heights showed a broad(7–16 km)and multi-modal distribution,with more than 40%of top heights appearing in the range of 9–10.5 km.Most of the cirrus cloud cases had thicknesses less than 3 km.Annual mean cirrus base and top heights were 8.89±1.65 km and 10.73±1.86 km,respectively.The annual mean thickness was～1.83±0.91 km.The mean LR for all cirrus cloud cases in our study was～25±17 sr,with a smooth seasonal variation.Approximately 70%of LRs fell within 18–40 sr, with a peak at 29 sr.No obvious relation between seasonal and annual mean LR and mid-cloud height was found.Large ranges in the magnitudes of cirrusσ(0.001–1.59 km?1)and cirrusτ(0.001–2.475)were observed.Annual mean cirrus cloudσandτwere 0.25±0.31 km?1and 0.34±0.33,respectively.Approximately12%ofthecirruscloudcaseswere sub-visible cirrus,43%were thin cirrus,and 45%were dense cirrus.Thicker cirrus clouds occurred more frequently duringthe summerthanin winter.Cirrus geometricaland optical propertiesderivedinthis studyaresimilartothosereportedin other studies using lasers to detect midlatitude cirrus clouds.

Acknowledgements.This study was supported by the Ministry of Science and Technology of China(Grant Nos.Change: 2013CB955802 to 2012AA120901),State Laboratory of Earth Surface Process and Resource Ecology,National Science Foundation of China(41175019),and the US Department of Energy(Grant Nos. DEFG0208ER64571and DE-SC0007171).The authors are grateful to Prof.Zhien WANG,University of Wyoming,for providing the cloud mask code.

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:Liu,J.J.,Z.Q.Li,Y.F.Zheng,andM.Cribb,2015:Cloud-basedistributionandcirrusproperties basedonmicropulse lidar measurements at a site in southeastern China.Adv.Atmos.Sci.,32(7),991–1004,

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(Received 09 August 2014;revised 11 November 2014;accepted 5 December 2014)

?Corresponding author:Zhanqing LI Email:11112010133@bnu.edu.cn

?Institute of Atmospheric Physics/Chinese Academy of Sciences,and Science Press and Springer-Verlag Berlin Heidelberg 2015